H81 Department
Water, Atmosphere and Environment H814
Institute of Meteorology Working Groups
Environmental Meteorology
ARSTM Project
ARSTM - Aerosols Remote Sensing and Transport Modelling
This project is funded by FWF, Lise-Meitner-Programme, Project number: M 2031-N29.
Staff: Camelia Talianu, Petra Seibert
Background:
Aerosols have a significant impact on air quality, and hence implicitly on human health, on Earth climate (both direct and indirect effects), on environment (water, land, vegetation) and on economical activities.
Aerosols are produced locally, with given properties; they are then transported over short- to long-distances, usually in turbulent movements. During transport, their physical and chemical properties can change due to chemical processes and meteorological conditions.
They can also mix with other aerosols, so more sources contribute to the aerosol budget in a given place. The lifetime of aerosols in the atmosphere is of the order of a week. Transport and dispersion of aerosols depend on aerosols' properties, on meteorological
conditions, and on surface properties.
Sources of aerosols are highly variable. As a consequence, the geographical distribution of aerosols is highly non-uniform and time-dependent.
To study the aerosols, precise measurement methods and large networks of instruments are needed. It is not possible to make continuous measurements covering all their trajectories, their sources are also not always known, therefore a detailed modelling of their
evolution is needed to provide values in intermediate locations, to identify their sources and to study their dispersion over large areas.
Lidar systems are the current state of the art active remote sensing instruments for aerosols measurements. They use elastic and inelastic (Raman) radiation scattering to provide time series of aerosol distributions and vertical profiles of the aerosols' optical coefficients; depolarization lidars additionally provide the depolarization profile, differentiating between spherical and non-spherical particles.
For passive remote sensing, the most advanced instruments are radiometers and photometers.
The most advanced ground-based observation networks set up to study the aerosols physical, chemical and optical properties:
- EARLINET - European aerosol lidar network provide the most extensive collection of ground-based data for the horizontal, vertical, and temporal distribution of aerosols over Europe.
- AERONET - federation of the ground-based passive remote sensing aerosol networks provides globally distributed observations of spectral aerosol optical depth (AOD), inversion products, and precipitable water in diverse aerosol regimes.
Numerical modelling of aerosols and their transport in space and time is an essential part of aerosol science. The modelling uses simulations to describe
how air pollutants disperse in the ambient atmosphere.
Overview:
Ground-based remote sensing measurements using lidars and the numerical modelling of aerosols play the central role in this project.
A quick analysis of the distribution of ground-based lidar stations used for aerosol measurements over Europe reveals a striking measuring gap in the southeastern part of Central Europe (Austria, Hungary, Czech Republic, Slovakia) between the four stations in Germany,
the five stations in Southeast Europe (Romania, Bulgaria, Greece, Cyprus) and the five stations in Italy.
For this project, data from ground-based remote sensing, in situ and satellite measurements covering a larger region centered on Austria, will be used:
- remote sensing data from EARLINET and AERONET from Romanian stations (Bucharest, Cluj-Napoca) and three German stations closest to Austria (Garmisch-Partenkirchen, Munich, Leipzig)
- MACC / CAMS products (integrating satellite data) from the European Copernicus Atmosphere Service, and CALIOP data
- in situ and remote sensing data from Austria.
In this project is used FLEXPART ("FLEXible PARTicle dispersion model") model. FLEXPART is a Lagrangian particle dispersion model designed for calculating the long-range and mesoscale transport,
diffusion, dry and wet deposition, and radioactive decay of air pollutants from point sources, such as after an accident in a nuclear power plant.
The original aspect of this project is the synergetic exploitation of the best available technologies (new generation of ground-based instruments, sensors and sunphotometers; state-of-the-art meteorological data and transport models; satellite imagery) with original methods for data analysis to determine aerosols' properties, their transport and their potential sources, resulting in significant improvements. These results are essential for the understanding of the direct and indirect effects of aerosols on climate, air quality and cloud-precipitation processes for the considered area.
Objectives:
- to use active remote sensing measurements together with satellite imagery and in situ data and new analysis methods in order to improve the identification of the aerosols types and the determination of their optical, microphysics and chemical properties,
- to define a new aerosol classification scheme
- to improve the capabilities of aerosol numerical modelling in FLEXPART using data from remote sensing measurements
- to show the benefits of including a hypothetical lidar station in the Austrian atmospheric research infrastructure, station eventually integrated in EARLINET
Activities:
- WP1: Analysis of aerosols over Austria - seasonal analysis and selected past periods
- WP2: Elaboration of an aerosol classification scheme based on optical and microphysics parameters
- WP3: Improving numerical modelling of aerosols in FLEXPART using remote sensing products
- WP4: Analysis of aerosols over Austria during a selected project period with improved FLEXPART
- WP5: Analysis of including a hypothetical lidar station for atmospheric studies in Vienna
Related Links:
EARLINET - European Aerosol Research Lidar Network to Establish an Aerosol Climatology
AERONET - Aerosol Robotic Network
ACTRIS - European Research Infrastructure for the observation of Aerosol, Clouds, and Trace gases.
CAMS - Copernicus Atmosphere Monitoring Service.
Results
Presentations:
- EGU General Assembly 2017 (Vienna, 23-28 April 2017): Characterization of long-range transport of aerosols over Austria
by Camelia Talianu and Petra Seibert (abstract) (poster)
- The 10th International Symposium on Tropospheric Profiling (ISTP10) (Fort Collins, Colorado, May 30 - June 2, 2017): Analysis of a case of sulfate aerosols over Austria
by Camelia Talianu and Petra Seibert (oral presentation)
- The 28th International Laser Radar Conference (Bucharest, 25-30 June 2017): Identification of long-range transport of aerosols over Austria using EARLINET lidar measurements
by Camelia Talianu (poster)
- European Aerosol Conference EAC 2017 (Zurich, Switzerland, Aug. 28 - Sept 1, 2017): Characterization of the aging process of smoke observed over Austria using organic carbon mixing ratio
by Camelia Talianu (abstract) (poster)
- EGU General Assembly 2018 (Vienna, 8-13 April 2018): Aerosol - ozone correlations for long-range aerosol transport over Austria
by Camelia Talianu and Petra Seibert (abstract) (poster)
- The 9th International Workshop on Sand/Duststorms and Associated Dustfall (22-24 May 2018, Tenerife, Spain): Impact of long-range transport of dust on in-situ measurements of particulate matter and ozone - case study: Austria
by Camelia Talianu and Petra Seibert (abstract) (poster)
List of peer-reviewed publications for project:
- C. Talianu and P. Seibert, "Characterization of long-range transport of aerosols over Austria," in Geophysical Research Abstracts, European Geosciences Union General Assembly 2017, Vienna, Austria, 2017, vol. 19, pp. EGU2017-10396 [Online]. Available:
https://meetingorganizer.copernicus.org/EGU2017/EGU2017-10396.pdf
- C. Talianu, "Identification of long-range transport of aerosols over Austria using EARLINET lidar measurements," EPJ Web Conf., vol. 176, p. 05053, Apr. 2018 [Online]. Available: https://www.epj-conferences.org/10.1051/epjconf/201817605053
- C. Talianu, "Characterization of the aging process of smoke observed over Austria using organic carbon mixing ratio," in European Aerosol Conference 2017, Zurich, Switzerland, 2017, vol. T205, p. T205N452 [Online]. Available:
http://www.gaef.de/EAC2017/EAC2017abstracts/T205/T205N452.pdf
- C. Talianu and P. Seibert, "Aerosol - ozone correlations for long-range aerosol transport over Austria," in Geophysical Research Abstracts, European Geosciences Union General Assembly 2018, Vienna, Austria, 2018, vol. 20, pp EGU2018-10028 [Online]. Available:
https://meetingorganizer.copernicus.org/EGU2018/EGU2018-10028.pdf
- C. Talianu and P. Seibert, "Impact of long-range transport of dust on in-situ measurements of particulate matter and ozone - case study: Austria," in The 9th International Workshop on Sand / Dust storm and Associated Dustfall, Tenerife, Spain, 2018 [Online].
Available: http://dustworkshop9.net/wp-content/uploads/2018/05/abstracts-dw9.pdf
- C. Talianu and P. Seibert, "Analysis of a case of sulfate aerosols over Austria," Manuscript under review for IEEE J. Sel. Top. Appl. Earth Obs. Remote Sens., vol. 12, no. 2, p. JSTARS-2018-00156, 2019.
- Nicolae, D., Vasilescu, J., Talianu, C., Binietoglou, I., Nicolae, V., Andrei, S., and Antonescu, B, "A Neural Network Aerosol Typing Algorithm Based on Lidar Data", Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-492, in review 2018.